Volume 49 (2006)

BASE CATALYZED SOL-GEL METHOD STARTING FROM TMOS FOR SYNTHESIS OF SILICA-PORPHYRIN NANOMATERIAL. FT-IR AND AFM CHARACTERIZATIONS
Pages 77-80
Corina Enache, Eugenia Fagadar-Cosma, Cecilia Savii, Raluca Gavrila

Abstract
Semiconducting materials such as silicon have contributed greatly to modern society. The use of photocurrent generating hybrid devices comprising organic molecules is now the state of art in this field. An experiment regarding porphyrin immobilization into silica matrix by using in situ sol-gel technique starting from TMOS is presented. The used para-hydroxyphenyl substituted porphyrin, namely: 5,10,15,20-tetrakis(4-hydroxyphenyl)-21H,23H-porphine, was isolated and purified by TLC, and column chromatography, after performing an Adler condensation reaction. The functional porphyrin and the silica-porphyrin hybrid material were monitored and characterized by 1H-NMR, FT-IR and UV-vis spectrometry. High-resolution imaging using atomic force microscopy (AFM) have been applied to directly observe the surface structures which are formed by immobilization of porphyrin on the surfaces.

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